Chemical solution deposition of single phase BiFeO3 thin films on transparent substrates
Journal article
Wang, Y., Zhang, M., Yue, Y., Zhang, H., Mahajan, A., Dunn, S. and Yan, H. (2022). Chemical solution deposition of single phase BiFeO3 thin films on transparent substrates. Solar RRL. https://doi.org/10.1002/solr.202200124
| Authors | Wang, Y., Zhang, M., Yue, Y., Zhang, H., Mahajan, A., Dunn, S. and Yan, H. |
|---|---|
| Abstract | The production of high quality BiFeO3 thin films on cost-effective transparent electrodes for visible light harvesting applications and devices remains a challenge. Here, we report the production of single-phase nanostructured BiFeO3 thin films via chemical solution deposition (CSD) on transparent conductive fluorine doped tin oxide FTO glass substrates. We show that the BiFeO3 is of high purity using a variety of analytical tools and that the as-obtained BiFeO3 thin films have a single grain single domain structure exhibiting ferroelectric switching under poling. The BiFeO3 samples show visible light absorption with a band gap of 2.7 eV under all processing conditions. By changing the annealing atmosphere it was possible to modify the photocurrent produced, which were (at 1.23 VNHE) 0.07 mA/cm2 (O2-annealed), 0.02 mA/cm2 (air-annealed) and 0.01 mA/cm2 (Ar-annealed). This indicates a change in the mobile carriers available. Our results show that it is possible to produce single phase BiFeO3 on a transparent conductive electrode system with controllable photoconductivity. |
| Keywords | Electrical and Electronic Engineering; Energy Engineering and Power Technology; Atomic and Molecular Physics, and Optics; Electronic, Optical and Magnetic Materials |
| Year | 2022 |
| Journal | Solar RRL |
| Publisher | Wiley |
| ISSN | 2367-198X |
| Digital Object Identifier (DOI) | https://doi.org/10.1002/solr.202200124 |
| Publication dates | |
| Online | 05 Apr 2022 |
| Publication process dates | |
| Accepted | 31 Mar 2022 |
| Deposited | 27 Apr 2022 |
| Publisher's version | License File Access Level Open |
| Accepted author manuscript | License File Access Level Controlled |
| License | http://onlinelibrary.wiley.com/termsAndConditions#vor |
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| Solar RRL - 2022 - Wang - Chemical solution deposition of single phase BiFeO3 thin films on transparent substrates.pdf | ||
| License: CC BY 4.0 | ||
| File access level: Open | ||
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